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A technique of measuring ion transfer between silver-nanoparticle and a single ionic liquid in solution is developed. We measure the free-energy change of ion transfer from the ionic liquid to the nanoparticles by electrochemistry and obtain the free-energy change as a function of the ion concentration in the ionic liquid. The ionic-liquid solution contained a silver nanoparticle with a diameter of approximately 10 nm as a liquid junction. The silver nanoparticles act as an electrochemical capacitor with a large capacitance, which results in an electrochemical cell with an extremely large Faraday response with a very low ion-transfer resistance. We successfully measure the transfer free-energy change of one Ag(+)-I(-) pair, by controlling the amount of Ag(+) contained in the liquid junction.cnxps.cmd.push(function () { cnxps({ playerId: '36af7c51-0caf-4741-9824-2c941fc6c17b' }).render('4c4d856e0e6f4e3d808bbc1715e132f6'); });
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